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- W4241356543 abstract "FeN4 moieties embedded in partially graphitized carbon are the most efficient platinum group metal free active sites for the oxygen reduction reaction in acidic proton-exchange membrane fuel cells. However, their formation mechanisms have remained elusive for decades because the Fe−N bond formation process always convolutes with uncontrolled carbonization and nitrogen doping during high-temperature treatment. Here, we elucidate the FeN4 site formation mechanisms through hosting Fe ions into a nitrogen-doped carbon followed by a controlled thermal activation. Among the studied hosts, the ZIF-8-derived nitrogen-doped carbon is an ideal model with well-defined nitrogen doping and porosity. This approach is able to deconvolute Fe−N bond formation from complex carbonization and nitrogen doping, which correlates Fe−N bond properties with the activity and stability of FeN4 sites as a function of the thermal activation temperature." @default.
- W4241356543 created "2022-05-12" @default.
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- W4241356543 date "2019-11-11" @default.
- W4241356543 modified "2023-10-17" @default.
- W4241356543 title "Thermally Driven Structure and Performance Evolution of Atomically Dispersed FeN <sub>4</sub> Sites for Oxygen Reduction" @default.
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- W4241356543 doi "https://doi.org/10.1002/ange.201909312" @default.
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