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- W4242281986 abstract "Temperature dependence of isotope effects in U(IV)-U(VI) exchange reaction was experimentally studied by means of redox chromatography using columns packed with anion exchange resin in the temperature range 87- 160°C (360–433 K). The experimentally observed isotopic separation coefficient, ε, was converted to the isotopic equilibrium constant, 1n K-εo, of the U(IV)-U(VI) exchange reaction with the aid of the experimentally measured ionic mole fractions of U(IV) and U(VI) in the resin phase and the aqueous solution phase. The plots of εo vs. 1/T led to the temperature dependence of εo=0.69/T-82/T2 , where the first term is due to the nuclear field effect (nuclear-electron interaction effect) and the second term is due to the molecular-vibration mass effect. The discussion is extended to the temperature dependence of the previously reported isotope effects in the U(III)-U(IV) electron exchange reaction, and the U(VI)-malate-complex ligand exchange reaction." @default.
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- W4242281986 date "2006-01-01" @default.
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- W4242281986 title "Temperature Dependence of Isotope Effects in Uranium Chemical Exchange Reactions" @default.
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- W4242281986 doi "https://doi.org/10.3327/jnst.43.400" @default.
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