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- W4242300926 abstract "Abstract Oxygen vacancy (Vo) on transition metal oxides plays a crucial role in determining their chemical/physical properties. Conversely, the capability to directly detect the changing process of oxygen vacancies (Vos) will be important to realize their full potentials in the related fields. Herein, with a novel synchronous illumination X‐ray photoelectron spectroscopy (SI‐XPS) technique, we found that the surface Vos (surf‐Vos) exhibit a strong selectivity for binding with the water molecules, and sequentially capture an oxygen atom to achieve the anisotropic self‐healing of surface lattice oxygen. After this self‐healing process, the survived subsurface Vos (sub‐Vos) promote the charge excitation from Ti to O atoms due to the enriched electron located on low‐coordinated Ti sites. However, the excessive sub‐Vos would block the charge separation and transfer to TiO 2 surfaces resulted from the destroyed atomic structures. These findings open a new pathway to explore the dynamic changes of Vos and their roles on catalytic properties, not only in metal oxides, but in crystalline materials more generally." @default.
- W4242300926 created "2022-05-12" @default.
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- W4242300926 date "2019-08-29" @default.
- W4242300926 modified "2023-10-16" @default.
- W4242300926 title "Direct Observation of Oxygen Vacancy Self‐Healing on TiO <sub>2</sub> Photocatalysts for Solar Water Splitting" @default.
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- W4242300926 doi "https://doi.org/10.1002/ange.201907954" @default.
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