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• W4243019235 abstract "Abstract. Five years (July 2007–June 2012) of CO tropospheric columns derived from the IASI hyperspectral infrared sounder onboard Metop-A are used to study the impact of fires on the concentrations of CO in the mid-troposphere. Following Chédin et al. (2005, 2008), who showed the existence of a daily tropospheric excess of CO2 quantitatively related to fire emissions, we show that tropospheric CO also displays a diurnal signal with a seasonality that is in very good agreement with the seasonal evolution of fires given by GFED3.1 (Global Fire Emission Database) emissions and MODIS (Moderate Resolution Imaging Spectroradiometer) burned area. Unlike daytime or nighttime CO fields, which mix local emissions with nearby emissions transported to the region of study, the day-night difference of CO allows to highlight the CO signal due to local fire emissions. A linear relationship is found in the whole tropical region between CO fire emissions from the GFED3.1 inventory and the diurnal difference of IASI CO (R2 ~ 0.6). Based on the specificity of the two main phases of the combustion (flaming vs. smoldering) and on the vertical sensitivity of the sounder to CO, the following mechanism is proposed to explain such a CO diurnal signal: at night, after the passing of IASI at 9.30 p.m. LT, a large amount of CO emissions from the smoldering phase is trapped in the boundary layer before being uplifted the next morning by natural and pyro-convection up to the free troposphere, where it is seen by IASI at 9.30 a.m. LT. The results presented here highlight the need for developing complementary approaches to bottom-up emissions inventories and for taking into account the specificity of both the flaming and smoldering phases of fire emissions in order to fully take advantage of CO observations." @default.
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• W4243019235 date "2014-10-17" @default.
• W4243019235 modified "2023-10-17" @default.
• W4243019235 title "Signature of tropical fires in the diurnal cycle of tropospheric CO as seen from Metop-A/IASI" @default.
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• W4243019235 doi "https://doi.org/10.5194/acpd-14-26003-2014" @default.
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