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• W4243199416 abstract "AbstractChiral Ga4L6 assembly Ga4(LN)6 encapsulates cationic iridium half-sandwich complexes that activate aldehyde C–H bonds to form chiral, strongly bound piano-stool complexes. Herein, we report the expanded scope of the larger Ga4(LP)6 host in mediating this transformation. The larger assembly significantly improves both the scope and the diastereoselectivity of this organometallic transformation generally, while substrate-specific interactions demonstrate that host size is an important, but not definitive, factor in determining diastereoselectivity.Keywords: supramolecular catalysisorganometallic chemistryC–H activation FundingThis research was supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231].Disclosure statementNo potential conflict of interest was reported by the authors." @default.
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• W4243199416 date "2016-01-29" @default.
• W4243199416 modified "2023-10-07" @default.
• W4243199416 title "Improved scope and diastereoselectivity of C–H activation in an expanded supramolecular host" @default.
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• W4243199416 doi "https://doi.org/10.1080/10610278.2015.1122196" @default.
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