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• W4243406332 endingPage "6686" @default.
• W4243406332 startingPage "6682" @default.
• W4243406332 abstract "Abstract Herein, we report on the first enantioselective and atom‐efficient catalytic one‐step dimerization method to selectively transform ω‐allenyl carboxylic acids into C 2 ‐symmetric 14‐ to 28‐membered bismacrolactones (macrodiolides). This convenient asymmetric access serves as an attractive route towards multiple naturally occuring homodimeric macrocyclic scaffolds and demonstrates excellent efficiency to construct the complex, symmetric core structures. By utilizing a rhodium catalyst with a modified chiral cyclopentylidene‐diop ligand, the desired diolides were obtained in good to high yields, high diastereoselectivity, and excellent enantioselectivity." @default.
• W4243406332 created "2022-05-12" @default.
• W4243406332 creator A5053761828 @default.
• W4243406332 creator A5067624195 @default.
• W4243406332 date "2018-05-03" @default.
• W4243406332 modified "2023-10-02" @default.
• W4243406332 title "Enantioselective Rhodium‐Catalyzed Dimerization of ω‐Allenyl Carboxylic Acids: Straightforward Synthesis of <i>C</i> ₂ ‐Symmetric Macrodiolides" @default.
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• W4243406332 doi "https://doi.org/10.1002/ange.201803369" @default.
• W4243406332 hasPublicationYear "2018" @default.
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