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- W4243607527 abstract "Abstract The higher‐order structures of semiconductor‐based photocatalysts play crucial roles in their physicochemical properties for efficient light‐to‐energy conversion. A novel perovskite SrTiO 3 mesocrystal superstructure with well‐defined orientation of assembled cubic nanocrystals was synthesized by topotactic epitaxy from TiO 2 mesocrystals through a facile hydrothermal treatment. The SrTiO 3 mesocrystal exhibits three times the efficiency for the hydrogen evolution of conventional disordered systems in alkaline aqueous solution. It also exhibits a high quantum yield of 6.7 % at 360 nm in overall water splitting and even good durability up to 1 day. Temporal and spatial spectroscopic observations revealed that the synergy of the efficient electron flow along the internal nanocube network and efficient collection at the larger external cubes produces remarkably long‐lived charges for enhanced photocatalysis." @default.
- W4243607527 created "2022-05-12" @default.
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- W4243607527 date "2017-04-06" @default.
- W4243607527 modified "2023-09-30" @default.
- W4243607527 title "Topotactic Epitaxy of SrTiO<sub>3</sub> Mesocrystal Superstructures with Anisotropic Construction for Efficient Overall Water Splitting" @default.
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- W4243607527 doi "https://doi.org/10.1002/ange.201702223" @default.
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