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- W4243897316 abstract "Existing methods for the covalent functionalization of nanoparticles rely on kinetically controlled reactions, and largely lack the sophistication of the preeminent oligonucleotide-based noncovalent strategies. Here we report the application of dynamic covalent chemistry for the reversible modification of nanoparticle (NP) surface functionality, combining the benefits of non-biomolecular covalent chemistry with the favorable features of equilibrium processes. A homogeneous monolayer of nanoparticle-bound hydrazones can undergo quantitative dynamic covalent exchange. The pseudomolecular nature of the NP system allows for the in situ characterization of surface-bound species, and real-time tracking of the exchange reactions. Furthermore, dynamic covalent exchange offers a simple approach for reversibly switching-and subtly tuning-NP properties such as solvophilicity.Ligandenaustausch: Der dynamisch‐kovalente Hydrazonaustausch innerhalb einer homogenen Monolage auf Goldnanopartikeln wird in Echtzeit untersucht. Die Einführung von geeignet funktionalisierten Aldehyd‐Austauscheinheiten ermöglicht die reversible Einstellung der Solvophilie der Nanopartikel. Die Methode könnte allgemein zur Nanopartikelmodifizierung angewendet werden.WILEY-VCH." @default.
- W4243897316 created "2022-05-12" @default.
- W4243897316 creator A5006463427 @default.
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- W4243897316 date "2015-01-14" @default.
- W4243897316 modified "2023-10-14" @default.
- W4243897316 title "Reversible Control of Nanoparticle Functionalization and Physicochemical Properties by Dynamic Covalent Exchange" @default.
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- W4243897316 doi "https://doi.org/10.1002/ange.201409602" @default.
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