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- W4243906172 abstract "A highly stereocontrolled, convergent total synthesis of kendomycin [(−)-TAN2162], an ansa-macrocyclic antibiotic, is reported. The key of the strategy is an unprecedented Tsuji–Trost macrocyclic etherification, followed by a transannular Claisen rearrangement to construct the 18-membered carbocyclic framework. The oxa-six- and five-membered rings were also stereoselectively constructed respectively by a cascade oxidative cyclization at an unfunctionalized benzylic position and using a one-pot epoxidation/5-exo-tet epoxide opening." @default.
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- W4243906172 date "2014-03-13" @default.
- W4243906172 modified "2023-09-27" @default.
- W4243906172 title "Total Synthesis of the Antibiotic Kendomycin: A Macrocyclization Using the Tsuji-Trost Etherification" @default.
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- W4243906172 doi "https://doi.org/10.1002/ange.201400305" @default.
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