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• W4244839763 endingPage "15380" @default.
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• W4244839763 abstract "The synthesis, structure, substitution chemistry, and optical properties of the gold-centered cubic monocationic cluster [Au@Ag8@Au6(C≡CtBu)12]+ are reported. The metal framework of this cluster can be described as a fragment of a body-centered cubic (bcc) lattice with the silver and gold atoms occupying the vertices and the body center of the cube, respectively. The incorporation of alkali metal atoms gave rise to [MnAg8−nAu7(C≡CtBu)12]+ clusters (n=1 for M=Na, K, Rb, Cs and n=2 for M=K, Rb), with the alkali metal ion(s) presumably occupying the vertex site(s), whereas the incorporation of copper atoms produced [CunAg8Au7−n(C≡CtBu)12]+ clusters (n=1–6), with the Cu atom(s) presumably occupying the capping site(s). The parent cluster exhibited strong emission in the near-IR region (λmax=818 nm) with a quantum yield of 2 % upon excitation at λ=482 nm. Its photoluminescence was quenched upon substitution with a Na+ ion. DFT calculations confirmed the superatom characteristics of the title compound and the sodium-substituted derivatives." @default.
• W4244839763 created "2022-05-12" @default.
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• W4244839763 date "2016-11-03" @default.
• W4244839763 modified "2023-09-26" @default.
• W4244839763 title "Site Preference in Multimetallic Nanoclusters: Incorporation of Alkali Metal Ions or Copper Atoms into the Alkynyl-Protected Body-Centered Cubic Cluster [Au₇Ag₈(C≡C^<i>t</i>Bu)₁₂]⁺" @default.
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• W4244839763 doi "https://doi.org/10.1002/ange.201609144" @default.
• W4244839763 hasPublicationYear "2016" @default.
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