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- W4244841805 abstract "Abstract Lithium hydride (LiH) has a strong effect on iron leading to an approximately 3 orders of magnitude increase in catalytic ammonia synthesis. The existence of lithium–iron ternary hydride species at the surface/interface of the catalyst were identified and characterized for the first time by gas‐phase optical spectroscopy coupled with mass spectrometry and quantum chemical calculations. The ternary hydride species may serve as centers that readily activate and hydrogenate dinitrogen, forming Fe‐(NH 2 )‐Li and LiNH 2 moieties—possibly through a redox reaction of dinitrogen and hydridic hydrogen (LiH) that is mediated by iron—showing distinct differences from ammonia formation mediated by conventional iron or ruthenium‐based catalysts. Hydrogen‐associated activation and conversion of dinitrogen are discussed." @default.
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- W4244841805 date "2017-06-12" @default.
- W4244841805 modified "2023-10-15" @default.
- W4244841805 title "The Formation of Surface Lithium-Iron Ternary Hydride and its Function on Catalytic Ammonia Synthesis at Low Temperatures" @default.
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- W4244841805 doi "https://doi.org/10.1002/ange.201703695" @default.
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