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- W4244889466 abstract "<a>The growth of three-dimensional covalent organic frameworks (3D COFs) with new topologies is still considered as a great challenge due to limited availability of high-connectivity building units. Here we report the design and synthesis of novel 3D triptycene-based COFs, </a><a></a><a>termed</a> JUC-568 and JUC-569, following the deliberate symmetry-guided design principle. By combining a triangular prism (6-connected) node with a planar triangle (3-connected) or another triangular prism node, the targeted COFs adopt unreported <b>ceq </b>or non-interpenetrated <b>acs</b> topology, respectively. <a>Both materials</a> show permanent porosity and impressive performance <a>in the adsorption of CO<sub>2</sub></a> (~ 98 cm<sup>3</sup>/g at 273 K and 1 bar), CH<sub>4</sub> (~ 48 cm<sup>3</sup>/g at 273 K and 1 bar), and especially H<sub>2</sub> (up to 274 cm<sup>3</sup>/g or 2.45 wt% at 77 K and 1 bar), which is <a>highest </a>among <a>porous organic materials</a> reported to date. This research thus provides a promising strategy for diversifying 3D COFs based on complex building blocks and promotes their <a></a><a>potential applications</a> <a>in</a><a></a><a> energy storage and environment-related field</a>s." @default.
- W4244889466 created "2022-05-12" @default.
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- W4244889466 date "2020-12-04" @default.
- W4244889466 modified "2023-09-29" @default.
- W4244889466 title "Three-Dimensional Triptycene-Based Covalent Organic Frameworks with ceq or acs Topology" @default.
- W4244889466 doi "https://doi.org/10.26434/chemrxiv.13311602" @default.
- W4244889466 hasPublicationYear "2020" @default.
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