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- W4245863939 abstract "Abstract Mesoporous carbon nitrides with C 3 N 5 and C 3 N 6 stoichiometries created a new momentum in the field of organic metal‐free semiconductors owing to their unique band structures and high basicity. Here, we report on the preparation of a novel graphitic microporous carbon nitride with a tetrazine based chemical structure and the composition of C 3 N 5.4 using ultra‐stable Y zeolite as the template and aminoguanidine hydrochloride, a high nitrogen‐containing molecule, as the CN precursor. Spectroscopic characterization and density functional theory calculations reveal that the prepared material exhibits a new molecular structure, which comprises two tetrazines and one triazine rings in the unit cell and is thermodynamically stable. The resultant carbon nitride shows an outstanding surface area of 130.4 m 2 g −1 and demonstrates excellent CO 2 adsorption per unit surface area of 47.54 μmol m −2 , which is due to the existence of abundant free NH 2 groups, basic sites and microporosity. The material also exhibits highly selective sensing over water molecules (151.1 mmol g −1 ) and aliphatic hydrocarbons due to its unique microporous structure with a high amount of hydrophilic nitrogen moieties and recognizing ability towards small molecules." @default.
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- W4245863939 date "2021-08-21" @default.
- W4245863939 modified "2023-10-16" @default.
- W4245863939 title "Microporous Carbon Nitride (C <sub>3</sub> N <sub>5.4</sub> ) with Tetrazine based Molecular Structure for Efficient Adsorption of CO <sub>2</sub> and Water" @default.
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- W4245863939 doi "https://doi.org/10.1002/ange.202108605" @default.
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