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- W4246173890 abstract "Abstract Inspired by the unique character of enzymes, we developed novel chiral SPO (secondary‐phosphine‐oxide) ligand (SPO‐Wudaphos) which can enter into both ion pair and H‐bond noncovalent interactions. The novel chiral SPO‐Wudaphos exhibited excellent results in the asymmetric hydrogenation of α‐methylene‐γ‐keto carboxylic acids, affording the chiral γ‐keto acids with up to over 99 % ee . A series of control experiments and DFT calculations were conducted to illustrate the critical roles of both the ion pair and H‐bond noncovalent interactions." @default.
- W4246173890 created "2022-05-12" @default.
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- W4246173890 date "2017-05-08" @default.
- W4246173890 modified "2023-10-16" @default.
- W4246173890 title "Enzyme-Inspired Chiral Secondary-Phosphine-Oxide Ligand with Dual Noncovalent Interactions for Asymmetric Hydrogenation" @default.
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- W4246173890 doi "https://doi.org/10.1002/ange.201701394" @default.
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