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• W4246361145 endingPage "8807" @default.
• W4246361145 startingPage "8803" @default.
• W4246361145 abstract "Regio- and stereoselective oxidative hydroxylation of achiral or chiral organic compounds mediated by synthetic reagents, catalysts, or enzymes generally leads to the formation of one new chiral center that appears in the respective enantiomeric or diastereomeric alcohols. By contrast, when subjecting appropriate achiral compounds to this type of CH activation, the simultaneous creation of two chiral centers with a defined relative and absolute configuration may result, provided that control of the regio-, diastereo-, and enantioselectivity is ensured. The present study demonstrates that such control is possible by using wild type or mutant forms of the monooxygenase cytochrome P450 BM3 as catalysts in the oxidative hydroxylation of methylcyclohexane and seven other monosubstituted cyclohexane derivatives." @default.
• W4246361145 created "2022-05-12" @default.
• W4246361145 creator A5050231254 @default.
• W4246361145 creator A5060598645 @default.
• W4246361145 creator A5068591898 @default.
• W4246361145 date "2014-03-03" @default.
• W4246361145 modified "2023-10-07" @default.
• W4246361145 title "Cytochrome P450 Catalyzed Oxidative Hydroxylation of Achiral Organic Compounds with Simultaneous Creation of Two Chirality Centers in a Single CH Activation Step" @default.
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• W4246361145 doi "https://doi.org/10.1002/ange.201310892" @default.
• W4246361145 hasPublicationYear "2014" @default.
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