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- W4246557635 abstract "Photolysis of H2S adsorbed on LiF(001) was studied by means of hydrogen Rydberg-atom time-of-flight spectroscopy. The H-atom translational energy distributions using 193.3 nm radiation showed three main features: a high energy channel attributed to H atoms escaping the surface without collisions (DIR); a vibrational progression from v=0 to v=5 [EL(v=0) and INEL(v>0)]; and a low energy channel attributed to multiple inelastic collisions [INEL(2)]. The vibrational progression can be attributed to two concurrent processes: the primary production of vibrationally excited SH in the dissociative event, and a secondary T→V energy transfer between the outgoing translationally hot H atom and a neighboring H2S(ad) molecule. The coverage dependence and angular distribution of the DIR, EL, and the INEL(v>0) channels has been used to define a minimum set of required H2S(ad) geometries." @default.
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- W4246557635 date "2000-07-08" @default.
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- W4246557635 title "Surface-aligned photochemistry: Photodissociation of H2S adsorbed on LiF(001) studied by Rydberg-atom time-of-flight spectroscopy" @default.
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- W4246557635 doi "https://doi.org/10.1063/1.481856" @default.
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