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- W4246561272 abstract "The self-assembly of trivalent lanthanide ions with ditopic organic spacers results in the formation of complex tiling patterns that mimic the structural motifs of quasi-periodic 2D materials. The assembly of <i>trans</i>-{LnI<sub>2</sub>}<sup>+</sup> nodes (Ln = Gd, Dy) with both closed-shell and anion radicals of 4,4'-bipyridine affords rare examples of Archimedean tessellations in a metal-organic framework. We furthermore demonstrate occurrence of sizable magnetic exchange interactions and slow relaxation of magnetization behaviour in a complex tessellation pattern. The implementation of Archimedean tessellations in lanthanide(III) coordination solids couriers a strategy to design elusive quasi<i>-periodic metal-organic frameworks with inimitable magnetic properties</i>" @default.
- W4246561272 created "2022-05-12" @default.
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- W4246561272 date "2021-05-05" @default.
- W4246561272 modified "2023-10-14" @default.
- W4246561272 title "Magnetic Archimedean Tessellations in Metal-Organic Frameworks" @default.
- W4246561272 doi "https://doi.org/10.26434/chemrxiv.14529090.v1" @default.
- W4246561272 hasPublicationYear "2021" @default.
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