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• W4246973054 endingPage "18308" @default.
• W4246973054 startingPage "18304" @default.
• W4246973054 abstract "Abstract An efficient Cp x Rh III ‐catalyzed enantioselective alkenyl C−H functionalization/[4+1] annulation of acryl amides and allenes is reported. The described transformation provides straightforward access to enantioenriched α,β‐unsaturated‐γ‐lactams bearing a quaternary stereocenter. The reaction operates under mild conditions, displays a broad functional‐group tolerance, and provides 2 H ‐pyrrol‐2‐ones with excellent selectivity of up to 97:3 er. Such scaffolds are frequently found in natural products and synthetic bioactive compounds and are of significant synthetic value. It is noteworthy that the allene serves as a one‐carbon unit in the [4+1]‐annulation." @default.
• W4246973054 created "2022-05-12" @default.
• W4246973054 creator A5018021290 @default.
• W4246973054 creator A5023363049 @default.
• W4246973054 creator A5091660912 @default.
• W4246973054 date "2019-10-28" @default.
• W4246973054 modified "2023-10-14" @default.
• W4246973054 title "Asymmetric Alkenyl C−H Functionalization by Cp ^x Rh ^III forms 2 <i>H</i> ‐Pyrrol‐2‐ones through [4+1]‐Annulation of Acryl Amides and Allenes" @default.
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