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- W4247296906 abstract "Abstract Polycyclic aromatic hydrocarbons (PAHs) are key components of organic electronics. The electronic properties of these carbon‐rich materials can be controlled through doping with heteroatoms such as B and N, however, few convenient syntheses of BN‐doped PAHs have been reported. Described herein is the rationally designed, two‐step syntheses of previously unknown ixene and BN‐doped ixene (B 2 N 2 ‐ixene), and their characterizations. Compared to ixene, B 2 N 2 ‐ixene absorbs longer‐wavelength light and has a smaller electrochemical energy gap. In addition to its single‐crystal structure, scanning tunneling microscopy revealed that B 2 N 2 ‐ixene adopts a nonplanar geometry on a Au(111) surface. The experimentally obtained electronic structure of B 2 N 2 ‐ixene and the effect of BN‐doping were confirmed by DFT calculations. This synthesis enables the efficient and convenient construction of BN‐doped systems with extended π‐conjugation that can be used in versatile organic electronics applications." @default.
- W4247296906 created "2022-05-12" @default.
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- W4247296906 date "2020-06-09" @default.
- W4247296906 modified "2023-10-13" @default.
- W4247296906 title "Unveiling 79‐Year‐Old Ixene and Its BN‐Doped Derivative" @default.
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- W4247296906 doi "https://doi.org/10.1002/ange.202004049" @default.
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