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• W4247307101 endingPage "638" @default.
• W4247307101 startingPage "624" @default.
• W4247307101 abstract "The results of a series of band-structure calculations for hypothetical forms of crystalline mercury with the fcc, bcc, sc, and diamond structures are applied to model the variation with density of $N({E}_{F})$, the density of states at the Fermi energy, in expanded liquid mercury. This quasicrystalline model is based on augmented-plane-wave (APW) energy-band calculations for each crystal structure with a fixed nearest-neighbor bond distance. The Fermi energy ${E}_{F}$ and $N(E)$ for each system are derived from a tight-binding fit to the APW results along symmetry lines in the Brillouin zone. The tight-binding wave functions are applied to decompose the total $N(E)$ into its $s$ and $p$ components, ${N}_{s}(E)$ and ${N}_{p}(E)$, respectively. It is found that the calculated variation of ${N}_{s}({E}_{F})$ with coordination provides a semiquantitative explanation for the observed variation of the Knight shift in liquid mercury with density. However, the corresponding variation of $N({E}_{F})$ with density fails to resolve the apparent contradiction between the Knight shift and the electronic transport properties in the strong scattering regime." @default.
• W4247307101 created "2022-05-12" @default.
• W4247307101 creator A5004214712 @default.
• W4247307101 creator A5046793602 @default.
• W4247307101 date "1977-07-15" @default.
• W4247307101 modified "2023-09-30" @default.
• W4247307101 title "Band model for the electronic structure of expanded liquid mercury" @default.
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• W4247307101 doi "https://doi.org/10.1103/physrevb.16.624" @default.
• W4247307101 hasPublicationYear "1977" @default.
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