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- W4247488468 abstract "<p>The broad scientific and technological importance of crystallization has led to significant research probing and rationalizing crystallization processes, particularly how nascent</p> <p>crystal phases appear. Previous work has generally neglected the possibility of the molecular-level dynamics of individual nuclei coupling to local structures (e.g., that of the nucleus and its</p> <p>surrounding environment). However, recent experimental work has conjectured that this can occur. Therefore, to address a deficiency in scientific understanding of crystallization, we have</p> <p>probed the nucleation of prototypical single and multi-component crystals (specifically, ice and mixed gas hydrates). Here, we establish that local structures can bias the evolution of nascent</p> <p>crystal phases on a nanosecond timescale by, for example, promoting the appearance or disappearance of specific crystal motifs, and thus reveal a new facet of crystallization behaviour.</p> <p>Analysis of the crystallization literature confirms that structural biases are likely present during crystallization processes beyond ice and gas hydrate formation. Moreover, we demonstrate that</p> <p>structurally-biased dynamics are a lens for understanding existing computational and experimental results while pointing to future opportunities.</p>" @default.
- W4247488468 created "2022-05-12" @default.
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- W4247488468 date "2018-10-02" @default.
- W4247488468 modified "2023-10-18" @default.
- W4247488468 title "Does Local Structure Bias How a Crystal Nucleus Evolves?" @default.
- W4247488468 doi "https://doi.org/10.26434/chemrxiv.7152296" @default.
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