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- W4247725885 abstract "Vitrification is observed under pressure at T = T sg from supercooled water. It is described in terms of enthalpy changes resulting from a competition between two liquids. In each, an additional enthalpy term is included in the Gibbs free energy of formation of superclusters at temperatures at which homogenous nucleation gives rise to ordered liquids upon supercooling. At the glass transition temperature T g ≅ 136.2 K, the two ordered liquids coexist when their enthalpy difference vanishes. A low-density amorphous phase of supercooled phase 3 and an ordered liquid phase 3 form at T g. A first-order transition occurs at T sg for 0.31 < P < 0.55 GPa and yields a high-density amorphous phase 3 whose T g is 0.65 T m. The ordered liquid phase 3 superheats at a temperature higher than the melting temperature T m and gives rise to a very high-density phase at P ≅ 0.95 GPa. A liquid-to-liquid transition exists at T LL ≅ 0.84335 T m for −0.149 < P < 0.176 GPa. Application of this phenomenology to other glass-forming liquids is also discussed." @default.
- W4247725885 created "2022-05-12" @default.
- W4247725885 creator A5018614490 @default.
- W4247725885 date "2021-02-01" @default.
- W4247725885 modified "2023-09-25" @default.
- W4247725885 title "Amorphous Ices" @default.
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- W4247725885 doi "https://doi.org/10.1002/9781118801017.ch3.14" @default.
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