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- W4247914741 abstract "The redox equilibrium of neptunium with nitric and nitrous acids was studied in 3 to 6M nitric acid solutions by 30vol% TBP-dodecane extraction. The equilibrium distribution ratio of neptunium was shown to be expressed by D=D6R/(1+R), where R is [Np(VI)]/[Np(V)] and D 6 the distribution ratio of pure Np(VI). To examine the dependence of the apparent concentration constant for the reaction on nitric acid concentration, the redox potentials of HNO3/HNO2 solutions were measured which revealed that the activity correction on H+, NO3 −, HNO2 and H2O was effective enough to give an ideal Nernst relationship for the potential of HNO3/HNO2. With using the activity coefficient quotient, Y=ys 2/(yuaw)1/2 (ys : stoichiometric activity coefficient of nitric acid, yu : activity coefficient of HNO2, aw : rational activity of water), the apparent concentration constant K app was shown to be expressed by K app=K mixY, where and log Y=-0.13, 0.02 and 0.28 for [HNO3]t=3, 4 and 6M, respectively." @default.
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- W4247914741 date "1995-01-01" @default.
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- W4247914741 title "Equilibrium of Nitrous Acid-Catalyzed Oxidation of Neptunium in Nitric Acid-TBP Extraction System" @default.
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- W4247914741 doi "https://doi.org/10.1080/18811248.1995.9731668" @default.
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