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- W4248295444 abstract "Abstract The high demand for electronic components from limited natural resources is forcing manufacturers to focus on thin-film technology but they are facing problems - limits of operation, uniformity of the films and expensive manufacturing tools. Chemistry can provide solutions to the last two problems with ease of manufacture and uniformity of two-dimensional materials retaining all functionalities within one single layer. Here, we present one such layered compound, [Co II (terpy)(H 2 O) 2 @Co II 2 (µ 2 -H 2 O) 3 {Ir III (ppy-COO) 3 } 2 ]·6H 2 O ( 1 ). Each charge-balanced layer is an anionic triple-ply holding [Co II (terpy)(H 2 O) 2 ] 2+ cations. Treating the crystals with warm acetone or by sonication breaks the weak interlayer supramolecular π-π and H-bonds leading to free standing single- and double layers (>30´30 µm 2 ). Each Co II (terpy)(H 2 O) 2 , at crystallographic positions 14.5 Å apart, behaves as a single-ion magnet (SIM). This is the first observation of periodic positioning of SIM shielded from their neighbours amounting to a staggering 350´10 12 Co II /in 2 capable of functioning as a 350 TeraBit/in 2 magnetic memory device." @default.
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- W4248295444 date "2020-10-19" @default.
- W4248295444 modified "2023-09-27" @default.
- W4248295444 title "Free Standing Large Area Metal-Organic Nanosheets Encapsulating Periodically Spaced Single-Ion Magnets" @default.
- W4248295444 doi "https://doi.org/10.21203/rs.3.rs-75308/v1" @default.
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