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• W4248466595 abstract "The study of manganese complexes as water-oxidation catalysts (WOCs) is of great interest because they can serve as models for the oxygen-evolving complex of photosystem II. In most of the reported Mn-based WOCs, manganese exists in the oxidation states III or IV, and the catalysts generally give low turnovers, especially with one-electron oxidants such as CeIV. Now, a different class of Mn-based catalysts, namely manganese(V)–nitrido complexes, were explored. The complex [MnV(N)(CN)4]2− turned out to be an active homogeneous WOC using (NH4)2[Ce(NO3)6] as the terminal oxidant, with a turnover number of higher than 180 and a maximum turnover frequency of 6 min−1. The study suggests that active WOCs may be constructed based on the MnV(N) platform." @default.
• W4248466595 created "2022-05-12" @default.
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• W4248466595 date "2015-02-26" @default.
• W4248466595 modified "2023-09-27" @default.
• W4248466595 title "Cerium(IV)-Driven Water Oxidation Catalyzed by a Manganese(V)-Nitrido Complex" @default.
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• W4248466595 doi "https://doi.org/10.1002/ange.201500507" @default.
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