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• W4248587232 endingPage "5063" @default.
• W4248587232 startingPage "5059" @default.
• W4248587232 abstract "2H-Azirines are easily synthesized from the corresponding ketones and, despite possessing a CN bond embedded in a strained three-membered cycle, they are sufficiently stable to be isolated, stored, and manipulated. 2H-Azirines can be regarded as valuable synthetic equivalents of alkenyl nitrenes, however, reactions capitalizing on the cyclic strain of the heterocyclic motif and involving the cleavage of the CN single bond remain surprisingly limited. A gold-catalyzed reaction that allows the formation of polysubstituted functionalized pyridines from easily accessible 2-propargyl 2H-azirine derivatives was developed. This transformation, which corresponds to an unprecedented intramolecular transfer of an alkenyl nitrene to an alkyne, proceeds with low catalyst loading, is efficient, and exhibits a high functional-group tolerance and a wide substrate scope." @default.
• W4248587232 created "2022-05-12" @default.
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• W4248587232 date "2014-04-08" @default.
• W4248587232 modified "2023-09-30" @default.
• W4248587232 title "Gold-Catalyzed Synthesis of Functionalized Pyridines by Using 2<i>H</i>-Azirines as Synthetic Equivalents of Alkenyl Nitrenes" @default.
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• W4248587232 doi "https://doi.org/10.1002/ange.201402470" @default.
• W4248587232 hasPublicationYear "2014" @default.
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