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- W4249444968 abstract "Abstract Domino processes initiated by intramolecular nucleopalladation of alkynes have been developed into powerful synthetic tools for the synthesis of functionalized heterocycles. However, a catalytic enantioselective version of this class of reactions remains scarce. We report herein that reaction of 2‐alkynylanilines with prochiral cyclopentenes in the presence of a catalytic amount of Pd(OAc) 2 , a chiral bidentate pyrox ligand and O 2 as terminal oxidant affords the structurally diverse indole‐cyclopentene conjugates bearing two stereocenters in a highly diastereo‐ and enantio‐selective manner. One of the products is converted to a heavily functionalized tetracyclic indolinone derivative." @default.
- W4249444968 created "2022-05-12" @default.
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- W4249444968 date "2021-02-17" @default.
- W4249444968 modified "2023-10-03" @default.
- W4249444968 title "Catalytic Enantioselective Aminopalladation–Heck Cascade" @default.
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- W4249444968 doi "https://doi.org/10.1002/ange.202016001" @default.
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