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- W4250993634 abstract "The synthesis and characterization of original NHC ligands based on an imidazo[1,5-a]pyridin-3-ylidene (IPy) scaffold functionalized with a flanking barbituric heterocycle is described as well as their use as tunable ligands for efficient gold-catalyzed C−N, C−O, and C−C bond formations. High activity, regio-, chemo-, and stereoselectivities are obtained for hydroelementation and domino processes, underlining the excellent performance (TONs and TOFs) of these IPy-based ligands in gold catalysis. The gold-catalyzed domino reactions of 1,6-enynes give rise to functionalized heterocycles in excellent isolated yields under mild conditions. The efficiency of the NHC gold 5Me complex is remarkable and mostly arises from a combination of steric protection and stabilization of the cationic AuI active species by ligand 1Me." @default.
- W4250993634 created "2022-05-12" @default.
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- W4250993634 date "2019-05-08" @default.
- W4250993634 modified "2023-10-18" @default.
- W4250993634 title "An Original L‐shape, Tunable N‐Heterocyclic Carbene Platform for Efficient Gold(I) Catalysis" @default.
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- W4250993634 doi "https://doi.org/10.1002/ange.201901090" @default.
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