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• W4251338823 startingPage "14267" @default.
• W4251338823 abstract "Abstract Selective oxidative cleavage of a CC bond offers a straightforward method to functionalize organic skeletons. Reported herein is the oxidative CC bond cleavage of ketone for CN bond formation over a cuprous oxide catalyst with molecular oxygen as the oxidant. A wide range of ketones and amines are converted into cyclic imides with moderate to excellent yields. In‐depth studies show that both α‐CH and β‐CH bonds adjacent to the carbonyl groups are indispensable for the CC bond cleavage. DFT calculations indicate the reaction is initiated with the oxidation of the α‐CH bond. Amines lower the activation energy of the CC bond cleavage, and thus promote the reaction. New insight into the CC bond cleavage mechanism is presented." @default.
• W4251338823 created "2022-05-12" @default.
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• W4251338823 date "2015-10-23" @default.
• W4251338823 modified "2023-09-30" @default.
• W4251338823 title "Cuprous Oxide Catalyzed Oxidative CC Bond Cleavage for CN Bond Formation: Synthesis of Cyclic Imides from Ketones and Amines" @default.
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• W4251338823 doi "https://doi.org/10.1002/ange.201508071" @default.
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