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- W4251372511 abstract "Abstract Although many methods are available for the synthesis of optically enriched monofluoromethyl secondary alcohols, synthesizing optically enriched monofluoromethyl tertiary alcohols remains a challenge. An efficient and easy‐to‐handle nucleophilic fluoromethylation protocol was developed. The current monofluoromethylation showed much higher facial selectivity than the corresponding difluoromethylation and proceeded via a different type of transition state. Excellent stereoselective control at the fluorinated carbon chiral center was found, an effect believed to be facilitated by the dynamic kinetic resolution of the chiral α‐fluoro carbanions." @default.
- W4251372511 created "2022-05-12" @default.
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- W4251372511 creator A5031890685 @default.
- W4251372511 creator A5047649448 @default.
- W4251372511 creator A5082644486 @default.
- W4251372511 date "2013-12-04" @default.
- W4251372511 modified "2023-10-18" @default.
- W4251372511 title "Stereoselective Nucleophilic Fluoromethylation of Aryl Ketones: Dynamic Kinetic Resolution of Chiral α-Fluoro Carbanions" @default.
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- W4251372511 doi "https://doi.org/10.1002/ange.201308484" @default.
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