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- W4252167768 abstract "A platinum-lined, flowing autoclave facility is used to investigate the solubility behavior of metallic nickel in hydrogenated ammonia and sodium hydroxide solutions between 175 and 315 °C. The solubility measurements were interpreted by means of an oxidative dissolution reaction followed by a sequence of Ni(II) ion hydrolysis reactions:andwhere n = 1 and 2. Gibbs energies associated with these reaction equilibria were determined from a least-squares analysis of the data. The extracted thermochemical properties (ΔfG0, ΔfH0 and S0) for Ni2+(aq), Ni(OH)+(aq) and Ni(OH)2(aq) were found to be consistent with those determined in a previous solubility study of NiO/Ni(OH)2 conducted in our laboratory. The thermodynamic basis of the Ni/NiO phase boundary in aqueous solutions is examined to show that Ni(s) is stable relative to NiO(s) in solutions saturated at 25 °C with 1 atm H2 for temperatures below 309 °C." @default.
- W4252167768 created "2022-05-12" @default.
- W4252167768 date "1995-12-01" @default.
- W4252167768 modified "2023-10-05" @default.
- W4252167768 title "Workshop on thermodynamic models and data for pure elements and other endmembers of solutions" @default.
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- W4252167768 doi "https://doi.org/10.1016/0364-5916(96)00005-3" @default.
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