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- W4252516897 abstract "Abstract Reported is a modular one‐step three‐component synthesis of tetrahydroisoquinolines using a Catellani strategy. This process exploits aziridines as the alkylating reagents, through palladium/norbornene cooperative catalysis, to enable a Catellani/Heck/aza‐Michael addition cascade. This mild, chemoselective, and scalable protocol has broad substrate scope (43 examples, up to 90 % yield). The most striking feature of this protocol is the excellent regioselectivity and diastereoselectivity observed for 2‐alkyl‐ and 2‐aryl‐substituted aziridines to access 1,3‐ cis ‐substituted and 1,4‐ cis ‐substituted tetrahydroisoquinolines, respectively. Moreover, this is a versatile process with high step and atom economy." @default.
- W4252516897 created "2022-05-12" @default.
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- W4252516897 date "2018-07-23" @default.
- W4252516897 modified "2023-09-25" @default.
- W4252516897 title "Modular One-Step Three-Component Synthesis of Tetrahydroisoquinolines Using a Catellani Strategy" @default.
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- W4252516897 doi "https://doi.org/10.1002/ange.201806780" @default.
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