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• W4253025149 endingPage "14299" @default.
• W4253025149 startingPage "14296" @default.
• W4253025149 abstract "Abstract A molybdenum–dithiolene–oxo complex was prepared as a model of some active sites of Mo/W‐dependent enzymes. The ligand, a quinoxaline–pyran‐fused dithiolene, mimics molybdopterin present in these active sites. For the first time, this type of complex was shown to be active as a catalyst for the photoreduction of protons with excellent turnover numbers (500) and good stability in aqueous/organic media and for the electroreduction of protons in acetonitrile with remarkable rate constants (1030 s −1 at −1.3 V versus Ag/AgCl). DFT calculations provided insight into the catalytic cycle of the reaction, suggesting that the oxo ligand plays a key role in proton exchange. These results provide a basis to optimize this new class of H 2 ‐evolving catalysts." @default.
• W4253025149 created "2022-05-12" @default.
• W4253025149 creator A5022444398 @default.
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• W4253025149 date "2015-09-25" @default.
• W4253025149 modified "2023-10-18" @default.
• W4253025149 title "A Bioinspired Molybdenum Complex as a Catalyst for the Photo‐ and Electroreduction of Protons" @default.
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• W4253025149 doi "https://doi.org/10.1002/ange.201505607" @default.
• W4253025149 hasPublicationYear "2015" @default.
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