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- W4253102015 abstract "Heteroatom- und sperrige Alkylsubstituenten erhöhen die Geschwindigkeit RhI-katalysierter (5+2)-Cycloadditionen von 1 drastisch. Ursache sind sterische Effekte, die die Vororganisation der Reaktanten erleichtern, und die Stabilisierung der Allylzwischenstufe durch (Hyper)konjugation mit den Substituenten. Methoxy- und Isopropyl-substituiertes 1 haben um 5 bzw. 7 kcal mol−1 niedrigere Aktivierungsenergien als das unsubstituierte Vinylcyclopropan. Supporting information for this article is available on the WWW under http://www.wiley-vch.de/contents/jc_2001/2008/z800420_s.pdf or from the author. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article." @default.
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- W4253102015 date "2008-05-13" @default.
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- W4253102015 title "Substituent Effects, Reactant Preorganization, and Ligand Exchange Control the Reactivity in RhI-Catalyzed (5+2) Cycloadditions between Vinylcyclopropanes and Alkynes" @default.
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- W4253102015 doi "https://doi.org/10.1002/ange.200800420" @default.
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