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- W4253699654 abstract "Abstract Single‐atom catalysts have attracted much attention. Reported herein is that regulating charge transfer of lattice oxygen atoms in serial single‐atom‐doped titania enables tunable hydrogen evolution reaction (HER) activity. First‐principles calculations disclose that the activity of lattice oxygen for the HER can be regularly promoted by substituting its nearest metal atom, and doping‐induced charge transfer plays an essential role. Besides, the realm of the charge transfer of the active site can be enlarged to the second nearest atom by creating oxygen vacancies, resulting in further optimization for the HER. Various single‐atom‐doped titania nanosheets were fabricated to validate the proposed model. Taking advantage of the localized charge transfer to the lattice atom is demonstrated to be feasible for realizing precise regulation of the electronic structures and thus catalytic activity of the nanosheets." @default.
- W4253699654 created "2022-05-12" @default.
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- W4253699654 date "2020-05-14" @default.
- W4253699654 modified "2023-10-17" @default.
- W4253699654 title "Regulating Charge Transfer of Lattice Oxygen in Single‐Atom‐Doped Titania for Hydrogen Evolution" @default.
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- W4253699654 doi "https://doi.org/10.1002/ange.202004510" @default.
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