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- W4254191811 abstract "Abstract Exploring an alternative anodic reaction to produce value‐added chemicals with high selectivity, especially integrated with promoted hydrogen generation, is desirable. Herein, a selective semi‐dehydrogenation of tetrahydroisoquinolines (THIQs) is demonstrated to replace the oxygen evolution reaction (OER) for boosting H 2 evolution reaction (HER) in water over a Ni 2 P nanosheet electrode. The value‐added semi‐dehydrogenation products, dihydroisoquinolines (DHIQs), can be selectively obtained with high yields at the anode. The controllable semi‐dehydrogenation is attributed to the in situ formed Ni II /Ni III redox active species. Such a strategy can deliver a variety of DHIQs bearing electron‐withdrawing/donating groups in good yields and excellent selectivities, and can be applied to gram‐scale synthesis. A two‐electrode Ni 2 P bifunctional electrolyzer can produce both H 2 and DHIQs with robust stability and high Faradaic efficiencies at a much lower cell voltage than that of overall water splitting." @default.
- W4254191811 created "2022-05-12" @default.
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- W4254191811 date "2019-08-01" @default.
- W4254191811 modified "2023-10-11" @default.
- W4254191811 title "Integrating Hydrogen Production with Aqueous Selective Semi‐Dehydrogenation of Tetrahydroisoquinolines over a Ni<sub>2</sub>P Bifunctional Electrode" @default.
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- W4254191811 doi "https://doi.org/10.1002/ange.201903327" @default.
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