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- W4254320912 abstract "Electrocatalytic conversion of carbon dioxide into high-value multicarbon (C2+) chemical feedstocks offers a promising avenue to liberate the chemical industry from fossil-resource dependence and eventually close the anthropogenic carbon cycle but is severely impeded by the lack of high-performance catalysts. To break the linear scaling relationship of intermediate binding and minimize the kinetic barrier of CO2 reduction reactions, ternary Cu–Au/Ag nanoframes were fabricated to decouple the functions of CO generation and C−C coupling, whereby the former is promoted by the alloyed Ag/Au substrate and the latter is facilitated by the highly strained and positively charged Cu domains. Thus, C2H4 production in an H-cell and a flow cell occurred with high Faradic efficiencies of 69±5 and 77±2 %, respectively, as well as good electrocatalytic stability and material durability. In situ IR and DFT calculations unveiled two competing pathways for C2H4 generation, of which direct CO dimerization is energetically favored." @default.
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- W4254320912 date "2020-11-27" @default.
- W4254320912 modified "2023-10-14" @default.
- W4254320912 title "Breaking the Linear Scaling Relationship by Compositional and Structural Crafting of Ternary Cu–Au/Ag Nanoframes for Electrocatalytic Ethylene Production" @default.
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- W4254320912 doi "https://doi.org/10.1002/ange.202012631" @default.
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