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• W4254482938 abstract "Abstract The reduced dimension perovskite including 2D perovskites are one of the most promising strategies to stabilize lead halide perovskite. A mixed‐cation 2D perovskite based on a steric phenyltrimethylammonium (PTA) cation is presented. The PTA‐MA mixed‐cation 2D perovskite of PTAMAPbI 4 can be formed on the surface of MAPbI 3 (PTAI‐MAPbI 3 ) by controllable PTAI intercalation by either spin coating or soaking. The PTAMAPbI 4 capping layer can not only passivate PTAI‐MAPbI 3 perovskite but also act as MA + locker to inhibit MAI extraction and significantly enhance the stability. The highly stable PTAI‐MAPbI 3 based perovskite solar cells exhibit a reproducible photovoltaic performance with a champion PCE of 21.16 %. Such unencapsulated devices retain 93 % of initial efficiency after 500 h continuous illumination. This steric mixed‐cation 2D perovskite as MA + locker to stabilize the MAPbI 3 is a promising strategy to design stable and high‐performance hybrid lead halide perovskites." @default.
• W4254482938 created "2022-05-12" @default.
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• W4254482938 date "2019-12-03" @default.
• W4254482938 modified "2023-10-16" @default.
• W4254482938 title "Steric Mixed‐Cation 2D Perovskite as a Methylammonium Locker to Stabilize MAPbI₃" @default.
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• W4254482938 doi "https://doi.org/10.1002/ange.201911518" @default.
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