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- W4255630574 abstract "Abstract Upon treatment with aryldiazonium salts, prenyl carbamates and ureas undergo redox‐neutral azocycloamination. In general, N‐aryl O‐prenyl carbamates cyclize in a photocatalytic reaction with visible light and an organic dye. With electron‐deficient diazonium salts, electronic matching with an electron‐rich N‐aryl substituent results in a reaction proceeding in the ground state, without either light or photocatalyst. Cyclic voltammetry suggests that this radical reaction is initiated by hydrogen‐atom abstraction mediated by an aryl radical, followed by a radical addition cascade and proton‐coupled hole propagation. The reaction proceeds at room temperature in short reaction times, and a range of functional groups is tolerated." @default.
- W4255630574 created "2022-05-12" @default.
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- W4255630574 date "2018-09-17" @default.
- W4255630574 modified "2023-09-30" @default.
- W4255630574 title "Transition Metal Free Cycloamination of Prenyl Carbamates and Ureas Promoted by Aryldiazonium Salts" @default.
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- W4255630574 doi "https://doi.org/10.1002/ange.201809323" @default.
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