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- W4256115265 abstract "Abstract A rhodium‐catalyzed intramolecular acetyl‐group transfer has been achieved through a “cut and sew” process. The challenge arises from the existence of different competitive pathways. Preliminary success has been achieved with unstrained enones that contain a biaryl linker. The use of an electron‐rich N‐heterocycilc carbene (NHC) ligand is effective to inhibit undesired β‐hydrogen elimination. Various 9,10‐dihydrophenanthrene derivatives can be prepared with excellent functional‐group compatibility. The 13 C‐labelling study suggests that the reaction begins with cleavage of the unstrained C−C bond, followed by migratory insertion and reductive elimination." @default.
- W4256115265 created "2022-05-12" @default.
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- W4256115265 date "2017-12-08" @default.
- W4256115265 modified "2023-10-08" @default.
- W4256115265 title "Intramolecular Acetyl Transfer to Olefins by Catalytic C−C Bond Activation of Unstrained Ketones" @default.
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- W4256115265 doi "https://doi.org/10.1002/ange.201711394" @default.
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