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- W4256482018 abstract "Abstract PGlue PZ , a pyrazoline (PZ)‐based fluorescent adhesive which can be generated spatiotemporally in living systems, was developed. Since PGlue PZ carries many guanidinium ion (Gu + ) pendants, it strongly adheres to various oxyanionic substrates through a multivalent salt‐bridge interaction. PGlue PZ is given by bioorthogonal photopolymerization of a Gu + ‐appended monomer (Glue TZ ), bearing tetrazole (TZ) and olefinic termini. Upon exposure to UV light, Glue TZ transforms into a nitrileimine (NI) intermediate (Glue NI ), which is eligible for 1,3‐dipolar polycycloaddition. However, Glue NI in aqueous media can concomitantly be deactivated into Glue WA by the addition of water, and the polymerization hardly occurs unless Glue NI is concentrated. We found that, even under high dilution, Glue NI is concentrated on oxyanionic substrates to a sufficient level for the polymerization, so that their surfaces can be point‐specifically functionalized with PGlue PZ by the use of a focused beam of UV light." @default.
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- W4256482018 date "2015-11-04" @default.
- W4256482018 modified "2023-10-16" @default.
- W4256482018 title "Photoinduced Bioorthogonal 1,3-Dipolar Poly-cycloaddition Promoted by Oxyanionic Substrates for Spatiotemporal Operation of Molecular Glues" @default.
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- W4256482018 doi "https://doi.org/10.1002/ange.201507987" @default.
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