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- W4256489495 abstract "Abstract Three component mobility controlling vinylic rotaxane crosslinkers with two radically polymerizable vinyl groups ( RC_R s) were synthesized to prove that the mobility of the components of the RC_R s plays a crucial role in determining the properties of rotaxane‐crosslinked polymers (RCPs). RC_R s (R=H, Me, or Et) were obtained from living ring‐opening polymerization. RCP_Et was prepared using RC_Et , which exhibits the lowest component mobility. The low component mobility is reflected in inferior mechanical strength and stretching ability in tensile stress tests compared to components with good (R=Me) and high (R=H) mobility. However, RCP_Et exhibited significantly higher stress and strain values than the corresponding covalently crosslinked polymers ( CCP_R s). These results indicate that a suitable component mobility substantially enhances the mechanical strength of RCPs. This behavior could serve as a guiding principle for the molecular design of advanced RCs." @default.
- W4256489495 created "2022-05-12" @default.
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- W4256489495 date "2019-01-25" @default.
- W4256489495 modified "2023-10-10" @default.
- W4256489495 title "A Guiding Principle for Strengthening Crosslinked Polymers: Synthesis and Application of Mobility‐Controlling Rotaxane Crosslinkers" @default.
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- W4256489495 doi "https://doi.org/10.1002/ange.201813439" @default.
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