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- W4280490504 abstract "This study focuses on the solar thermo-catalytic methane decomposition for hydrogen and C2-hydrocarbons production in an indirectly-irradiated tubular solar reactor. The proposed concept is based on a two-step process encompassing the CH4 decomposition into C2-hydrocarbons and hydrogen at high temperatures, followed by the decomposition of C2-hydrocarbons into solid carbon and hydrogen at lower temperatures (both steps can be catalyzed using metal catalysts). Methane decomposition represents an attractive approach for CO2-free hydrogen production using concentrated solar energy as the high-temperature process heat source. A series of solar experiments were conducted to investigate the effect of the addition of gas quenching operation at the downstream of the heating section in the reactor for the production of C2-hydrocarbons and hydrogen from methane at high-temperature (1,400 °C). The results showed a slight improvement of C2H2 yield in the case without catalyst but CH4 conversion and H2 yield decreased significantly in this case. Conversely, a significant improvement of C2H2 yield was observed when adding catalyst (W strips) without reducing the CH4 conversion." @default.
- W4280490504 created "2022-05-22" @default.
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- W4280490504 date "2022-01-01" @default.
- W4280490504 modified "2023-09-26" @default.
- W4280490504 title "Enhanced production of C2-hydrocarbons and hydrogen from catalytic methane decomposition in a tubular reactor heated by concentrated solar energy" @default.
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- W4280490504 doi "https://doi.org/10.1063/5.0086250" @default.
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