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- W4280491569 abstract "Electro-assisted adsorption (EAA) is an environmentally friendly, effective and economical method for phosphate removal, and its electrosorption capacity is strongly dependent on the electrode material. Herein, we fabricated a MOF-derived hierarchically porous carbon (ZrMC) electrode for the selective electrosorption of phosphate. At 1 V condition, the ZrMC electrode demonstrated a high removal rate of 2.08 mg g−1 min−1 within 40 min, and the maximum electrosorption capability of 163.30 mg g−1 according to Langmuir isothermal model. The excellent performance for phosphate electrosorption was attributed to the hierarchically porous structure, excellent conductivity, and abundant active centers. The electrosorption data was well-fitted with the pseudo-second-order kinetics model. Interestingly, by applying reversed voltage, the ZrMC electrode exhibited an outstanding desorption capacity of 88.33% after ten cycles. Finally, the corresponding electrosorption mechanism was comprehensively clarified by both the Fourier transform infrared spectrometer (FTIR) and X-ray photoelectron spectrometer (XPS) measurements. Our work implies that the ZrMC electrode has a promising potential for highly efficient removal and recovery of phosphate." @default.
- W4280491569 created "2022-05-22" @default.
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- W4280491569 date "2022-08-01" @default.
- W4280491569 modified "2023-10-12" @default.
- W4280491569 title "Efficient electro-assisted adsorption/desorption of phosphate on MOF-derived hierarchically porous carbon electrode" @default.
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- W4280491569 doi "https://doi.org/10.1016/j.jclepro.2022.132262" @default.
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