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• W4280492267 endingPage "23636" @default.
• W4280492267 startingPage "23624" @default.
• W4280492267 abstract "Optically induced magnetic resonances (OMRs) are highly tunable scattering states that cannot be reproduced in systems that only support electric resonances, such as in metals, lossy, or low-index materials. Despite offering unique scattering and coupling behavior, the study of OMRs in thin films has been limited by synthesis and simulation constraints. We report on the absorption and scattering response of OMR-based thin films composed of monodisperse crystalline silicon nanoparticles synthesized using a scalable nonthermal plasma growth technique and tractable simulation framework. The synthesis is solvent and ligand free, ensuring minimal contamination, and crystalline particles form with high yield and a narrow size distribution at close to room temperature. Using a scalable high-throughput deposition method, we deposit random particle films, without the need of a solid host matrix, showing near complete blackbody absorption at the collective OMR. This is achieved using 70% less material than an optimized antireflective-coated crystalline silicon thin film. The film exhibits strongly directional forward scattering with very low reflectivity, thus giving rise to angle- and polarization-insensitive antireflection properties across the visible spectrum. We find that, while commonly used effective medium models cannot capture the optical response, a modified effective medium accounting for multipole resonances and interparticle coupling shows excellent agreement with experiment. The effective permittivity and permeability are written in a mode and cluster resolved form, providing useful insight into how individual resonances and nanoparticle clusters affect the overall film response. Electric and magnetic-mode coupling show dramatically different behavior, resulting in uniquely different spectral broadening." @default.
• W4280492267 created "2022-05-22" @default.
• W4280492267 creator A5000398736 @default.
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• W4280492267 creator A5079355304 @default.
• W4280492267 creator A5079969926 @default.
• W4280492267 creator A5082887836 @default.
• W4280492267 date "2022-05-12" @default.
• W4280492267 modified "2023-10-18" @default.
• W4280492267 title "Broadband, Angle- and Polarization-Invariant Antireflective and Absorbing Films by a Scalable Synthesis of Monodisperse Silicon Nanoparticles" @default.
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• W4280492267 doi "https://doi.org/10.1021/acsami.2c03263" @default.
• W4280492267 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35549027" @default.
• W4280492267 hasPublicationYear "2022" @default.
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