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- W4280492918 abstract "Reported herein is the discovery of a diastereoselective indole-dearomative Cope rearrangement. A suite of minor driving forces promote dearomatization: (i) steric congestion in the starting material, (ii) alkylidene malononitrile and stilbene conjugation events in the product, and (iii) an unexpected intramolecular π–π* stack on the product side of the equilibrium. The key substrates are rapidly assembled from simple starting materials, resulting in many successful examples. The products are structurally complex and bear vicinal stereocenters generated by the dearomative Cope rearrangement. They also contain a variety of functional groups for interconversion to complex architectures." @default.
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- W4280492918 date "2022-05-16" @default.
- W4280492918 modified "2023-09-25" @default.
- W4280492918 title "Diastereoselective Indole-Dearomative Cope Rearrangements by Compounding Minor Driving Forces" @default.
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- W4280492918 doi "https://doi.org/10.1021/acs.orglett.2c01381" @default.
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