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• W4280497896 abstract "Photocatalysis is facing huge challenges especially the separation and efficient utilization of photocarriers. Herein, we report that a ternary hollow core-shell photocatalyst is synthesized by template and self-assembled method. The experimental results show that the electron separation efficiency and utilization efficiency are significantly improved, not only because the ternary hollow core-shell structure spatially separates the oxidation area MnOx from the reduction area Co-MOF, but also because lots of emergent electrons are stored in Co-MOF as an electronic library, contributing to the formation of surface polarization to support the requirement call from the CoP quantum dots (QDs) as active-sites. It's the first report that the effectively separated electron-rich and electron-poor microelectronic states of the tunable Co-MOF promotes electron utilization by affecting the storage capacity of the electron library promoting photocatalytic hydrogen production. The tests show that Mn@Cd-CoP QDs/MCN (35.31 mmol/h/g), Mn@Cd-CoP QDs/BCN (23.69 mmol/h/g) and Mn@Cd-CoP QDs (11.08 mmol/h/g) have the better hydrogen production performances, which is about 38 times, 26 times and 12 times higher than CdS (0.9244 mmol/h/g), respectively. The pioneering exploration about the ternary hollow core-shell structure bonded with MOFs materials with abundant CoP QDs will open up a new perspective to design high-performance for solar-chemical energy conversion." @default.
• W4280497896 created "2022-05-22" @default.
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• W4280497896 date "2022-10-01" @default.
• W4280497896 modified "2023-09-23" @default.
• W4280497896 title "Microelectronic structure changes electron utilization: Core-shell structure catalysts with electron library and quantum dots for photocatalytic hydrogen production" @default.
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• W4280497896 doi "https://doi.org/10.1016/j.jcis.2022.05.048" @default.
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