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- W4280508732 abstract "Herein, we demonstrate that the surface anchoring of black phosphorus quantum dots (BPQDs) and bulk iron-doping in W18 O49 nanowires significantly promotes the photocatalytic activity toward N2 fixation into NH3 . More specifically, a NH3 production rate of up to 187.6 μmol g-1 h-1 could be achieved, nearly one order of magnitude higher than that of pristine W18 O49 (18.9 μmol g-1 h-1 ). Comprehensive experiments and density-functional theory calculations reveal that Fe-doping could enhance the reducing ability of photo-generated electrons by decreasing the work function and elevating the defect band (d-band) centers. Additionally, the surface BPQDs anchoring could facilitate the N2 adsorption/activation owing to the increased adsorption energy and advantaged W-P dimer bonding-mode. Therefore, synergizing the surface BPQD anchoring and bulk Fe-doping remarkably enhanced the photocatalytic activity of W18 O49 nanowires for NH3 production." @default.
- W4280508732 created "2022-05-22" @default.
- W4280508732 creator A5017021792 @default.
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- W4280508732 date "2022-06-07" @default.
- W4280508732 modified "2023-10-14" @default.
- W4280508732 title "Anchoring Black Phosphorus Quantum Dots on Fe‐Doped W<sub>18</sub>O<sub>49</sub> Nanowires for Efficient Photocatalytic Nitrogen Fixation" @default.
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- W4280508732 doi "https://doi.org/10.1002/anie.202204271" @default.
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