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- W4280542012 abstract "The construction of heterogeneous frustrated Lewis pairs (FLPs) with performance comparable to or surpassing the homogeneous counterparts in H2 activation is a long-standing challenge. Herein, sterically hindered Lewis acid (B center) and Lewis base (N center) sites were anchored within the rigid lattice of highly crystalline hexagonal boron nitride (h-BN) scaffolds. The active sites were created via precision defect regulation during the molten-salt-involved (NaNH2 and NaBH4) h-BN construction procedure. The as-afforded h-BN scaffolds achieved highly efficient H2/D2 activation and dissociation under ambient pressure via FLP-like behavior, and attractive catalytic efficiency in hydrogenation reactions surpassing the current heterogeneous analogues." @default.
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- W4280542012 date "2022-05-19" @default.
- W4280542012 modified "2023-09-29" @default.
- W4280542012 title "Defect-Regulated Frustrated-Lewis-Pair Behavior of Boron Nitride in Ambient Pressure Hydrogen Activation" @default.
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- W4280542012 doi "https://doi.org/10.1021/jacs.2c00343" @default.
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