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• W4280570388 abstract "Fabricating high performance thermosets through the formation of specific nanostructures via suitable design of block copolymer has become a new trend in recent years. While the correspondence between nanostructures and block copolymer was rarely reported, especially in the field of reaction-induced microphase separation. In our work, three linear diblock copolymers poly(ε-caprolactone)- block -polystyrene (PCL-PS) with similar molecular weights but different compositions were successfully synthesized. Then, they were implanted into the epoxy matrix to prepare nanostructured composites. The effects of PCL-PS concentration and composition on the organization and transformation of nanostructures in resin matrix were systemically investigated. Meanwhile, the relationship between macro properties of epoxy composites and the morphology of nanostructures was also researched. We hope readers can get some theoretical advice from our work for constructing specific nanostructures in epoxy composites depending on the self-assembly method of block copolymer. • Three linear diblock copolymers PCL-PS with similar molecular weights but different compositions were successfully synthesized. • Three linear diblock copolymers were incorporated into the epoxy matrix to prepare nanostructured composites by self-assembly method. • The reaction-induced microphase separation can be changed by adjusting the structural composition of the block copolymer, and it can be clearly observed by SEM. • When a small amount of block copolymer is added, it can bring about a great improvement in mechanical properties and an obviously increase in T g ." @default.
• W4280570388 created "2022-05-22" @default.
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• W4280570388 date "2022-07-01" @default.
• W4280570388 modified "2023-10-16" @default.
• W4280570388 title "Nanostructure transformation in epoxy/block copolymer composites with good mechanical properties" @default.
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• W4280570388 doi "https://doi.org/10.1016/j.reactfunctpolym.2022.105299" @default.
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